One needs to do a :
 $ systemctl daemon-reload

After putting the file there.

The error is
/lib/systemd/system/ntp.service:6] Unknown lvalue '+ EnvironmentFile' in 
section 'Service'

Removing the 'plus-sign' won't fix it.


[OT but important bread-crumbs for others...]

The systemd-timesyncd.service works out of the box - no need to do anything but enable it in systemd - but if you need your own time server it fixes nothing. And if you want to use systemd-timesyncd.service and point it at your own time server you need to edit /etc/systemd/timesyncd.conf
 - the keyword Servers needs a Capital 's' and the s at the end.

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